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All you need to do is to log into your MSFT account and add your wife Microsoft account to your account as family since you can have up to 6 users on the family account/plan and each user can access on 5 computers. If she does not have a Microsoft account, you need to create one for her and add it as a family on your plan. Once this is done, you need to log in on her desktop by launching either excel or Microsoft word and then go to account and login with her information and that should give her access to Office 365 Family plan and all the features that comes with it.
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